I think I could be here all day naming my faves honestly. There are so many wonderful shows that I couldn't truly settle on a title or two. Like with my fave Seiyuus I tend to change my top fave animes often. So I'll just name a few of my most recent faves.
Kiddy Grade, Ef - A Tale of Melodies, Seitokai Yakuindomo, Zero no Tsukaima (all three seasons), Claymore, Fate/Stay Night.